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• Table (5)
• Contents (5)

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  personenkennziffer
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  K. Wu
  false
  1
  L. Wang
  false
  2
  S. Colón-Rodríguez
  false
  3
  Gerd-Uwe Flechsig
  https://www.hs-coburg.de/personen/prof-dr-gerd-uwe-flechsig/
  true
  4
  T. Wang
  false
  

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Amidyl Radical Directed Remote Allylation of Unactivated sp3 C-H Bonds by Organic Photoredox Catalysis

The development of visible-light-mediated allylation of unactivated sp3 C-H bonds is reported. The remote allylation was directed by the amidyl radical, which was generated by photocatalytic fragmentation of a pre-functionalized amide precursor. Both aromatic and aliphatic amide derivatives could successfully deliver the remote C-H allylation products in good yields. A variety of electron deficient allyl sulfone systems could be used as d-carbon radical acceptor.

Wu, K.; Wang, L.; Colón-Rodríguez, S.; Flechsig, Gerd-Uwe; Wang, T. (2019): Amidyl Radical Directed Remote Allylation of Unactivated sp3 C-H Bonds by Organic Photoredox Catalysis. Angewandte Chemie (International ed. in English) 2019 58 (6), S. 1774–1778. DOI: 10.1002/anie.201811004

https://www.hs-coburg.de/publikation/2712-amidyl-radical-directed-remote-allylation-of-unactivated-sp3-c-h-bonds-by-organic-photoredox-catalysis/